Density-controlled and seedless growth of laterally bridged ZnO nanorod for UV photodetector applications

Ming Yueh Chuang, Hsin-Chieh Yu, Yan Kuin Su*, Chih Hung Hsiao, Tsung Hsien Kao, Chien Sheng Huang, Yu Chun Huang, Jeng Je Tsai, San Lein Wu

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

14 Scopus citations

Abstract

This study develops a density-controlled and seedless growth method for laterally bridged ZnO nanorods from Au electrode for use in metal-semiconductor- metal photodetector fabrication. The effect of pre-annealing process on suppressing vertical ZnO nanorods is systematically investigated by atomic force microscopy and scanning electron microscopy. The pre-annealing process is demonstrated to have direct influence on controlling vertical/lateral ZnO nanorod density and morphology. Interlaced and density-controlled ZnO nanorods with approximate single-crystalline structure can be directly grown from the side wall of pre-annealed Au electrode fingers without seed-layer. Through pre-annealing process, dark-current can be decreased from 4.99 × 10 -4 to 7.28 × 10-7 A with an applied voltage of 1 V. Highly dense lateral ZnO nanorod-based photodetectors produce remarkable responsivity of 7.01 × 103 A/W and UV/visible rejection ratio of 281.21. Moreover, a high internal photoconductive gain (10 4-105) exists in the fabricated photodetectors. For a given bandwidth of 10 kHz and 1 V applied bias, the noise equivalent power of photodetectors with 0, 10, and 20 min pre-annealing periods are estimated to be 3.58 × 10-13, 6.78 × 10-13, and 4.86 × 10-13 W, and correspond to normalized detectivity of 1.85 × 1012, 1.17 × 1012, and 1.99 × 1012 cm Hz0.5 W-1, respectively. This result may be attributed to internal photoconductive gain mechanism and high-density bridged ZnO nanorods. Our approach provides a simple and controllable method to fabricate high-performance ultraviolet photodetectors.

Original languageEnglish
Pages (from-to)810-819
Number of pages10
JournalSensors and Actuators, B: Chemical
Volume202
DOIs
StatePublished - 31 Oct 2014

Keywords

  • Hydrothermal growth
  • Internal photoconductivity gain
  • Laterally bridged
  • UV photodetector
  • ZnO nanorod

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