Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe1/2Nb1/2)O3-PbMO3 (M-Ti, Zr) multiferroic solid solutions

I. P. Raevski; V. V. Titov; V. V. Laguta; M. Marysko; S. P. Kubrin; Haydn Chen; C. C. Chou; A. V. Blazhevich; S. I. Raevskaya; D. A. Sarychev; T. A. Minasyan; L. A. Pustovaya; I. N. Zakharchenko; M. A. Malitskaya

doi:10.1080/00150193.2015.994989

Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe_1/2Nb_1/2)O₃-PbMO₃ (M-Ti, Zr) multiferroic solid solutions

I. P. Raevski^*, V. V. Titov, V. V. Laguta, M. Marysko, S. P. Kubrin, Haydn Chen, C. C. Chou, A. V. Blazhevich, S. I. Raevskaya, D. A. Sarychev, T. A. Minasyan, L. A. Pustovaya, I. N. Zakharchenko, M. A. Malitskaya

^*Corresponding author for this work

International College of Semiconductor Technology

Research output: Contribution to journal › Article › peer-review

19 Scopus citations

Abstract

Some peculiar features of magnetic x,T-phase diagram of (1-x)PbFe_1/2Nb_1/2O₃-xPbTiO₃ system at x ≈ 0.1 have been ascribed previously to the change of the lattice symmetry from rhombohedral to tetragonal or to the decrease of the lattice parameter with x. We carried out structural, dielectric, magnetization, and Mossbauer studies of (1-x)PbFe_1/2Nb_1/2O₃-xPbZrO₃ system, where the symmetry remains rhombohedral, while the lattice parameter increases with x. However, the magnetic x,T-phase diagram of (1-x)PbFe_1/2Nb_1/2O₃-xPbZrO₃ appeared to be very similar to that of (1-x)PbFe_1/2Nb_1/2O₃-xPbTiO₃. Anomalies of composition dependence of magnetic phase transition temperatures at x ≈ 0.1 are supposed to be due to the percolation phase transition.

Original language	English
Pages (from-to)	20-30
Number of pages	11
Journal	Ferroelectrics
Volume	475
Issue number	1
DOIs	https://doi.org/10.1080/00150193.2015.994989
State	Published - 25 Jan 2015

Keywords

Ferroelectric
lead iron niobate
multiferroic
phase transition diffusion
spin glass

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Raevski, I. P., Titov, V. V., Laguta, V. V., Marysko, M., Kubrin, S. P., Chen, H., Chou, C. C., Blazhevich, A. V., Raevskaya, S. I., Sarychev, D. A., Minasyan, T. A., Pustovaya, L. A., Zakharchenko, I. N., & Malitskaya, M. A. (2015). Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe_1/2Nb_1/2)O₃-PbMO₃ (M-Ti, Zr) multiferroic solid solutions. Ferroelectrics, 475(1), 20-30. https://doi.org/10.1080/00150193.2015.994989

Raevski, I. P. ; Titov, V. V. ; Laguta, V. V. ; Marysko, M. ; Kubrin, S. P. ; Chen, Haydn ; Chou, C. C. ; Blazhevich, A. V. ; Raevskaya, S. I. ; Sarychev, D. A. ; Minasyan, T. A. ; Pustovaya, L. A. ; Zakharchenko, I. N. ; Malitskaya, M. A. / Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe_1/2Nb_1/2)O₃-PbMO₃ (M-Ti, Zr) multiferroic solid solutions. In: Ferroelectrics. 2015 ; Vol. 475, No. 1. pp. 20-30.

@article{90fec35d577643f2a2075d6943ddae0c,

title = "Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe1/2Nb1/2)O3-PbMO3 (M-Ti, Zr) multiferroic solid solutions",

abstract = "Some peculiar features of magnetic x,T-phase diagram of (1-x)PbFe1/2Nb1/2O3-xPbTiO3 system at x ≈ 0.1 have been ascribed previously to the change of the lattice symmetry from rhombohedral to tetragonal or to the decrease of the lattice parameter with x. We carried out structural, dielectric, magnetization, and Mossbauer studies of (1-x)PbFe1/2Nb1/2O3-xPbZrO3 system, where the symmetry remains rhombohedral, while the lattice parameter increases with x. However, the magnetic x,T-phase diagram of (1-x)PbFe1/2Nb1/2O3-xPbZrO3 appeared to be very similar to that of (1-x)PbFe1/2Nb1/2O3-xPbTiO3. Anomalies of composition dependence of magnetic phase transition temperatures at x ≈ 0.1 are supposed to be due to the percolation phase transition.",

keywords = "Ferroelectric, lead iron niobate, multiferroic, phase transition diffusion, spin glass",

author = "Raevski, {I. P.} and Titov, {V. V.} and Laguta, {V. V.} and M. Marysko and Kubrin, {S. P.} and Haydn Chen and Chou, {C. C.} and Blazhevich, {A. V.} and Raevskaya, {S. I.} and Sarychev, {D. A.} and Minasyan, {T. A.} and Pustovaya, {L. A.} and Zakharchenko, {I. N.} and Malitskaya, {M. A.}",

year = "2015",

month = jan,

day = "25",

doi = "10.1080/00150193.2015.994989",

language = "English",

volume = "475",

pages = "20--30",

journal = "Ferroelectrics",

issn = "0015-0193",

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Raevski, IP, Titov, VV, Laguta, VV, Marysko, M, Kubrin, SP, Chen, H, Chou, CC, Blazhevich, AV, Raevskaya, SI, Sarychev, DA, Minasyan, TA, Pustovaya, LA, Zakharchenko, IN & Malitskaya, MA 2015, 'Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe_1/2Nb_1/2)O₃-PbMO₃ (M-Ti, Zr) multiferroic solid solutions', Ferroelectrics, vol. 475, no. 1, pp. 20-30. https://doi.org/10.1080/00150193.2015.994989

Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe_1/2Nb_1/2)O₃-PbMO₃ (M-Ti, Zr) multiferroic solid solutions. / Raevski, I. P.; Titov, V. V.; Laguta, V. V.; Marysko, M.; Kubrin, S. P.; Chen, Haydn; Chou, C. C.; Blazhevich, A. V.; Raevskaya, S. I.; Sarychev, D. A.; Minasyan, T. A.; Pustovaya, L. A.; Zakharchenko, I. N.; Malitskaya, M. A.

In: Ferroelectrics, Vol. 475, No. 1, 25.01.2015, p. 20-30.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe1/2Nb1/2)O3-PbMO3 (M-Ti, Zr) multiferroic solid solutions

AU - Raevski, I. P.

AU - Titov, V. V.

AU - Laguta, V. V.

AU - Marysko, M.

AU - Kubrin, S. P.

AU - Chen, Haydn

AU - Chou, C. C.

AU - Blazhevich, A. V.

AU - Raevskaya, S. I.

AU - Sarychev, D. A.

AU - Minasyan, T. A.

AU - Pustovaya, L. A.

AU - Zakharchenko, I. N.

AU - Malitskaya, M. A.

PY - 2015/1/25

Y1 - 2015/1/25

N2 - Some peculiar features of magnetic x,T-phase diagram of (1-x)PbFe1/2Nb1/2O3-xPbTiO3 system at x ≈ 0.1 have been ascribed previously to the change of the lattice symmetry from rhombohedral to tetragonal or to the decrease of the lattice parameter with x. We carried out structural, dielectric, magnetization, and Mossbauer studies of (1-x)PbFe1/2Nb1/2O3-xPbZrO3 system, where the symmetry remains rhombohedral, while the lattice parameter increases with x. However, the magnetic x,T-phase diagram of (1-x)PbFe1/2Nb1/2O3-xPbZrO3 appeared to be very similar to that of (1-x)PbFe1/2Nb1/2O3-xPbTiO3. Anomalies of composition dependence of magnetic phase transition temperatures at x ≈ 0.1 are supposed to be due to the percolation phase transition.

AB - Some peculiar features of magnetic x,T-phase diagram of (1-x)PbFe1/2Nb1/2O3-xPbTiO3 system at x ≈ 0.1 have been ascribed previously to the change of the lattice symmetry from rhombohedral to tetragonal or to the decrease of the lattice parameter with x. We carried out structural, dielectric, magnetization, and Mossbauer studies of (1-x)PbFe1/2Nb1/2O3-xPbZrO3 system, where the symmetry remains rhombohedral, while the lattice parameter increases with x. However, the magnetic x,T-phase diagram of (1-x)PbFe1/2Nb1/2O3-xPbZrO3 appeared to be very similar to that of (1-x)PbFe1/2Nb1/2O3-xPbTiO3. Anomalies of composition dependence of magnetic phase transition temperatures at x ≈ 0.1 are supposed to be due to the percolation phase transition.

KW - Ferroelectric

KW - lead iron niobate

KW - multiferroic

KW - phase transition diffusion

KW - spin glass

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U2 - 10.1080/00150193.2015.994989

DO - 10.1080/00150193.2015.994989

M3 - Article

AN - SCOPUS:84925248468

VL - 475

SP - 20

EP - 30

JO - Ferroelectrics

JF - Ferroelectrics

SN - 0015-0193

IS - 1

ER -

Comparative studies of ferroelectric and magnetic phase transitions in Pb(Fe_1/2Nb_1/2)O₃-PbMO₃ (M-Ti, Zr) multiferroic solid solutions

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Keywords

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